Download e-book for iPad: Advances in Organometallic Chemistry, 7 by F G A Stone; Robert West

By F G A Stone; Robert West

ISBN-10: 0080580084

ISBN-13: 9780080580081

ISBN-10: 0120311070

ISBN-13: 9780120311071


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Additional info for Advances in Organometallic Chemistry, 7

Example text

M. Gomberg, and others, in their early and epochal work establishing the existence of trivalent carbon in triarylmethyls, put to great use the synthetic possibilities of organometallic compounds for the preparation of the necessary hexaarylethanes. The organic chemist still needed experimental support for the existence of free alkyl radicals in the interpretation of many organic reactions in which there was little doubt of the intermediate participation of such alkyl radicals. It remained for F.

It was found that the position of absorption attributed to the Si-Si bond chromophore shifted to longer wavelengths, and a considerable increase in molar absorptivities occurred with the four compounds. Thus the conjugation existing in the unsubstituted More Than One-Half Century of Organometallic Chemistry 43 diphenylsilane has been increased due to the substituents in the benzene rings, the least change occurring with the most electronegative substituent. Along the lines just mentioned, we synthesized, with I.

Growing out of the catenation work was the development with C. Smith concerned with the preparation and examination of the completely symmetrical and highly branched types. One representative of this group is tetrakis(trimethylsily1)silane. SiMes I MesSi-Si-SiMes I SiMes As might be expected in such types, the compounds tend to be highmelting, with high volatility, and enhanced thermal stability. A novel and very reactive type directly derivable from the parent type, is tris(trimethy1sily1)silyllithium.

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Advances in Organometallic Chemistry, 7 by F G A Stone; Robert West

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